Focused Laser Beam Research Articles

Formation of Highly Tunable Periodic Plasmonic Structures on Gold Films Using Direct Laser Writing

AbstractDirect laser writing method is a promising technique for the large‐scale and cost‐effective fabrication of periodic nanostructure arrays exciting hybrid lattice plasmons. This type of electromagnetic mode manifests a narrow and deep resonance peak with a high dispersion whose precise controllability is crucial for practical applications in photonic devices. Here, the formation of differently shaped gold nanostructures using the direct laser writing method on Au layers of different thicknesses is presented. The resonance peak is demonstrated to be highly dependent on the shape of the structures in the array, thus its position in the spectra, as well as the quality, can be additionally modulated by changing the morphology. The shape of the structure and the resonance itself pertain not only on the laser pulse energy but also on the grating period. This overlapping effect occurring at distances smaller than the diameter of the focused laser beam is studied in detail. By taking advantage of the highly controllable plasmonic resonance, the fabricated gratings open up new opportunities for applications in sensing.

Fast-speed algorithm to compute tight focusing of laser beams: Effectiveness of circularly polarized vortex beam series as a mathematical basis

Fast-speed algorithm to compute tight focusing of laser beams: Effectiveness of circularly polarized vortex beam series as a mathematical basis

Using Laser Point Scanning Thermography for Quality Monitoring of Products Made of Composite Materials

Introduction. Control of the presence of subsurface defects in products from composite materials is necessary for verification of products after release from production and in the process of operation. Aim of the Study. The purpose of the presented work is to estimate the parameters of subsurface defects using local laser thermography, suitable for quality control of both small objects and suspicious areas of large objects with curved surfaces. Materials and Methods. The laboratory setup on which this work was carried out includes a robotic arm, a COX CG640 thermal imager and a 3 W laser. The method was tested on a fiberglass sample with introduced delamination defect simulations located at different depths below the surface. By means of computer modeling rational parameters of thermographic control were selected, providing reliable detection of the defect at a depth of up to 3 mm under the surface of the composite sample. Results. Numerical modeling of surface temperature field induced by moving focused laser beam was carried out using COMSOL software package. It showed that laser beam with 3 W power moving at 5 mm/s provided the thermal contrast sufficient to detect the defects at the depth up to 3 mm. The obtained experimental data are in satisfactory agreement with numerical modeling both qualitatively and quantitatively. Experimental data were used to construct a regression model for determining defect depth based on the maximal thermal contrast and the time interval between heating and the contrast maximum. Discussion and Conclusion. The results obtained in this work allow us to propose a technique for detecting defects in fiberglass plastics and estimating their depth. The coefficient of determination for the obtained regression model was found to be equal to 0.95, and the mean square error of the metric was no more than 0.016 mm2. The use of a robotic arm to scan objects will make it possible to investigate objects with complex curved surfaces.

KrF laser-driven shock tube: Realization and first experiments

We report on the first implementation of a miniature laser-driven shock tube (LDST) of 5 × 5 mm cross section and 50-mm length for generating and studying strong shock waves (SW) and hypersonic gas flows with M > 10. Operation of the LDST is based on the acceleration of a thin CH-film by ablative plasma pressure produced when the film is irradiated by high-energy UV pulse of the GARPUN KrF laser (100 J & 100-ns). The film serves as a piston that pushes a SW in the gas filling the LDST. An optical system based on a multi-element prism raster provides focusing of KrF laser beam into 7 × 7 mm square spot with 100 J/cm2 energy fluence (1 GW/cm2 intensity) with inhomogeneity ∼3 % across the LDST aperture. It is expected that the LDST with KrF laser driver can be an effective tool for studying hydrodynamic phenomena, such as hydrodynamic instabilities and transition to a turbulence, hypersonic gas flow around bodies, reflection and cumulation of strong SW.

Nonlinear Photodetector Based on InSe p–n Homojunction for Improving Spatial Imaging Resolution

AbstractAn efficient nonlinear photodetector (NLPD) is demonstrated with quadratic response based on a few‐layer InSe p–n homojunction, which is beneficial from the strong second harmonic generation (SHG) process in InSe and effective harvest of photocarriers actuated by the high‐quality homojunction. The NLPD can sense light with photon energy smaller than InSe's electronic bandgap because the SHG process in InSe doubles the frequency of incident light, extending InSe's photodetection wavelength range to 1750 nm. The InSe p–n homojunction, which is electrostatically doped by two split back gates, presents a rectification ratio exceeding 106 with a dark current down to 2 pA and a high normalized responsivity of 0.534 A W−2 for the telecom‐band pulsed light at 1550 nm. The photocurrents of the SHG‐assisted photodetection have a quadratic dependence on the optical powers, making the NLPD highly sensitive to light intensity variation with improved spatial resolution. As examples, the NLPD is employed to precisely determine the localization point of a focused laser beam waist and implement spatial imaging with an improved resolution compared with the linear photodetector. These features highlight the potential of the proposed NLPD in developing advanced optical sensing and imaging systems.

Enhanced terahertz emission in a large-area photoconductive antenna through an array of tightly packed sapphire fibers

Experimental observation of the enhanced terahertz (THz) emission in a large-area photoconductive antenna-emitter (LAE), boosted by an array of cylindrical sapphire-fiber-based microlenses, is reported. The observed enhancement is achieved, thanks to the sharp focusing of a pump laser beam near the semiconductor surface, for which the high-refractive-index sapphire lenses are used. We predict numerically and confirm experimentally a considerable enhancement in the emitted THz spectral power for such a sapphire-fiber-coupled LAE, as compared to an ordinary one with an equal electrode topology. In fact, a ≃8.5-fold THz power boost is achieved, resulting in a +9.3 dB increase in the dynamic range. The results of our findings can be used to improve the performance of large-area THz devices, aimed at meeting the demands of rapidly developed THz spectroscopy, imaging, sensing, and exposure technologies.

Three-Dimensional Optothermal Manipulation of Light-Absorbing Particles in Phase-Change Gel Media.

Rational manipulation and assembly of discrete colloidal particles into architected superstructures have enabled several applications in materials science and nanotechnology. Optical manipulation techniques, typically operated in fluid media, facilitate the precise arrangement of colloidal particles into superstructures by using focused laser beams. However, as the optical energy is turned off, the inherent Brownian motion of the particles in fluid media impedes the retention and reconfiguration of such superstructures. Overcoming this fundamental limitation, we present on-demand, three-dimensional (3D) optical manipulation of colloidal particles in a phase-change solid medium made of surfactant bilayers. Unlike liquid crystal media, the lack of fluid flow within the bilayer media enables the assembly and retention of colloids for diverse spatial configurations. By utilizing the optically controlled temperature-dependent interactions between the particles and their surrounding media, we experimentally exhibit the holonomic microscale control of diverse particles for repeatable, reconfigurable, and controlled colloidal arrangements in 3D. Finally, we demonstrate tunable light-matter interactions between the particles and 2D materials by successfully manipulating and retaining these particles at fixed distances from the 2D material layers. Our experimental results demonstrate that the particles can be retained for over 120 days without any change in their relative positions or degradation in the bilayers. With the capability of arranging particles in 3D configurations with long-term stability, our platform pushes the frontiers of optical manipulation for distinct applications such as metamaterial fabrication, information storage, and security.

The Advantages and Disadvantages of Using Structured High-Order but Single Laguerre–Gauss LGp0 Laser Beams

Most laser applications are based on the focusing of a Gaussian laser beam (GLB). When the latter is subject to a phase aberration such as the optical Kerr effect (OKE) or spherical aberration (SA), it is recognised that the focusing performance of the GLB is degraded. In this paper, it is demonstrated that high-order radial Laguerre–Gauss LGp0 beams are more resilient than the GLB when subject to the OKE or SA. This opens up opportunities to replace with advantages the usual GLB with a high-order LGp0 beam for some applications.

Structured Excitation Energy Transfer: Tracking Exciton Diffusion below Sunlight Intensity.

With the increasing demand for new materials for light-harvesting applications, spatiotemporal microscopy techniques are receiving increasing attention as they allow direct observation of the nanoscale diffusion of excitons. However, the use of pulsed and tightly focused laser beams generates light intensities far above those expected under sunlight illumination, leading to photodamage and nonlinear effects that seriously limit the accuracy and applicability of these techniques, especially in biological or atomically thin materials. In this work, we present a novel spatiotemporal microscopy technique that exploits structured excitation in order to dramatically decrease the excitation intensity, up to 10,000-fold when compared with previously reported spatiotemporal photoluminescence microscopy experiments. We tested our method in two different systems, reporting the first exciton diffusion measurement at illumination conditions below sunlight, both considering average power and peak exciton densities in an organic photovoltaic sample (Y6), where we tracked the excitons for up to five recombination lifetimes. Next, nanometer-scale energy transport was directly observed for the first time in both space and time in a printed monolayer of the light-harvesting complex 2 from purple bacteria.

Optofluidic-based deformability cytometry: Characterizing erythrocyte elasticity and assessing storage quality

Erythrocyte elasticity is an inherent, label-free marker for both physiological and pathological changes in erythrocytes, serving as a criterion for assessing the quality and suitability of stored blood. Although varieties of cell elasticity measurement techniques have been proposed, a small sample, non-contact, and continuous method is still in need. This article introduces an optofluidic-based deformability cytometry (O-DC) for characterizing erythrocyte elasticity, combining non-contact optical force with microfluidic technology. A tightly focused laser beam optically traps an erythrocyte, and the flow force induces cell deformation, allowing for elasticity characterization through force-dependent elongation. The O-DC technique offers high accuracy and desirable throughput for cell elasticity characterization, facilitated by quasi-static stretching and continuous cell delivery. The characterization throughput of O-DC is ∼3 cells per second at a flow rate of 30 μL/h and a laser power of 200 mW. Fresh erythrocytes exhibit measured elastic strains of 15.4–27.8% across flow rates of 10–30 μL/h, with an estimated elastic modulus of 2.6±0.3 μN/m. Using O-DC, the elasticity trend of erythrocytes stored for 0–6 weeks was analyzed, with their average elastic modulus increasing from 2.6±0.3 μN/m to 6.1±0.8 μN/m as the storage time increased. Our study highlights the potential of O-DC in clinical diagnostics and biomechanical research applications.

Temperature Relaxation in Glass-Forming Materials under Local Fast Laser Excitations during Laser-Induced Microstructuring

The ability to control the temperature distribution T(t,r) and the rate of temperature change Rt,r inside glasses is important for their microstructuring. The lattice temperature is considered at time t, exceeding the electron–phonon thermalization time, and at a distance r from the center of the model spherical heating zone. In order to describe thermal excitations, the heat capacity of glasses must be considered as a function of time due to its long-term relaxation. A method for the analytical calculation of T(t,r) and R(t,r) for glasses with dynamic heat capacity cdyn(t) is proposed. It is shown that during laser microstructuring, the local cooling rate −R(t,r) significantly depends on the time dispersion of cdyn(t). It has been established that at the periphery of the model heating zone of the laser beam focus, the local cooling rate can reach more than 1011 K/s. Strong cooling rate gradients were found at the periphery of the heating zone, affecting the microstructure of the material. This effect is significantly enhanced by the time dispersion of cdyn(t). The effect associated with this time dispersion is significant, even well above the glass transition temperature Tg, since even short relaxation times of the dynamic heat capacity cdyn(t) are significant.

Probe beam deflection technique with liquid immersion for fast mapping of thermal conductance

Frequency-domain probe beam deflection (FD-PBD) is an experimental technique for measuring thermal properties that combines heating by a modulated pump laser and measurement of the temperature field via thermoelastic displacement of the sample surface. In the conventional implementation of FD-PBD, the data are mostly sensitive to the in-plane thermal diffusivity. We describe an extension of FD-PBD that introduces sensitivity to through-plane thermal conductance by immersing the sample in a dielectric liquid and measuring the beam deflection created by the temperature field of the liquid. We demonstrate the accuracy of the method by measuring (1) the thermal conductivity of a 310 nm thick thermally grown oxide on Si, (2) the thermal boundary conductance of bonded interface between a 3C-SiC film and a single crystal diamond substrate, and (3) the thermal conductivities of several bulk materials. We map the thermal boundary conductance of a 3C-SiC/diamond interface with a precision of 1% using a lock-in time constant of 3 ms and dwell time of 15 ms. The spatial resolution and maximum probing depth are proportional to the radius of the focused laser beams and can be varied over the range of 1–20 μm and 4–80 μm, respectively, by varying the 1/e2 intensity radius of the focused laser beams from 2 to 40 μm. FD-PBD with liquid immersion thus enables fast mapping of spatial variations in thermal boundary conductance of deeply buried interfaces.

Optical Tweezers Apparatus Based on a Cost-Effective IR Laser-Hardware and Software Description.

Optical tweezers (OT), or optical traps, are a device for manipulating microscopic objects through a focused laser beam. They are used in various fields of physical and biophysical chemistry to identify the interactions between individual molecules and measure single-molecule forces. In this work, we describe the development of a homemade optical tweezers device based on a cost-effective IR diode laser, the hardware, and, in particular, the software controlling it. It allows us to control the instrument, calibrate it, and record and process the measured data. It includes the user interface design, peripherals control, recording, A/D conversion of the detector signals, evaluation of the calibration constants, and visualization of the results. Particular stress is put on the signal filtration from noise, where several methods were tested. The calibration experiments indicate a good sensitivity of the instrument that is thus ready to be used for various single-molecule measurements.

Enhancement of optical levitation with hyperbolic metamaterials

The tightly focused laser beam in an optical trap has become a useful tool for many recent research areas. The momentum change in the photon-stream path of incident laser beam induces radiation force that enables trapping and manipulating mesoscopic micron-sized objects. In this study, we report the first analytical demonstration of optical trapping and levitation with radiation pressure on a transparent micron-sized spherical object made of hyperbolic metamaterial (HMM). The optical radial and axial forces acting on dielectric and HMM spherical particles are calculated using ray-optics approximation, assuming an optical levitation trapping setup. We compared the net force acting on the two objects, finding that the net radiation force exerted towards HMM particle is enhanced in the axial direction: The optical force enhancement in the HMM particle is more than ~ 8 times stronger compared to the induced force on the conventional dielectric particle with the corresponding material parameters. Besides, a better performance in the radial stabilization is observed for the HMM particle in comparison with the dielectric case, at which some oscillations and unstable saturation locations for the radial stabilization is monitored for TEM00 beam incidence. Furthermore, “zero-force” paths where radial stabilization of the HMM particle exists are also obtained for both TEM00 and TEM01∗\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$TEM_{01}^{*}$$\\end{document} laser beam incidences. Such phenomenon does not occur for particles of only dielectric and only metal material, which can be considered as another superiority of the proposed HMM particle.

Laser-Induced Transformations in Thermally Evaporated Thin TlInSe2 Films Studied by Raman Spectroscopy

TlInSe2 films with thickness from 10 to 200 nm were thermally evaporated on silicon and silicate glass substrates. Micro-Raman spectra measured at a moderate excitation (532 nm, 4 kW/cm2) confirm the amorphous character of the films. Narrow features revealed in the spectra at an excitation power density of 40 kW/cm2 show the evidence for the formation of TlInSe2 , TlSe, and In2Se3 crystallites in the laser spot. For thin (10–30 nm) films, the rod-shaped TlInSe2 crystallites are shown to be oriented within the film plane. The crystallite formation is governed by the thermal effect of the tightly focused laser beam.

Using Optical Tweezers Combined with Total Internal Reflection Microscopy to Study Interactions Between the ER and Golgi in Plant Cells.

Optical tweezers have been used to trap and micro-manipulate several biological specimens ranging from DNA, macromolecules, organelles, to single-celled organisms. Using a combination of the refraction and scattering of laser light from a focused laser beam, refractile objects are physically captured and can be moved within the surrounding media. The technique is routinely used to determine biophysical properties such as the forces exerted by motor proteins. Here, we describe how optical tweezers combined with total internal reflection fluorescence microscopy (TIRF) can be used to assess physical interactions between organelles, more specifically the ER and Golgi bodies in plant cells.

Effect of Laser Process Loops on the Hole Diameter and Hole Formation of Laser Micro Drilling on TC4

Laser micro drilling stands as a precise manufacturing method that employs a focused laser beam to craft accurate, small holes within a diverse array of materials. Its applications span across vital industries like aerospace, medical, and electronics, playing a pivotal role in creating components like fuel injectors, medical implants, and microelectronics. Within this context, a notable challenge emerges in obtaining a refined surface finish during laser micro drilling. This study delves into the impact of a laser loop, a crucial parameter, on the surface quality of TC4, also known as Ti6Al4V—an aerospace staple. Employing a Conventional Fiber Laser with a peak output of 30 W, the experiment meticulously directs the laser beam onto the TC4 surface via a microscope objective lens. The drilling process unfolds in controlled conditions, mitigating external variables such as temperature and humidity. Assessment of drilled hole surfaces transpires through both light and 3D microscopes. Interestingly, holes subjected to higher laser power and increased laser loop rates demonstrate enhanced surface smoothness. In essence, this inquiry demonstrates the substantial influence of laser loop on TC4’s surface finish during laser micro drilling. Elevating the laser loop factor leads to heightened surface refinement and diminished roughness in drilled holes. It was found that the diameter entry of the micro-holes was increased by 61% - 89.35% and the diameter exit of the micro-holes also increased by 55.55% - 62.79%. The outcomes of this investigation offer valuable insights for refining the laser micro drilling process to achieve premium surface quality on TC4 and comparable materials. As such, these findings extend guidance for optimal laser loop settings in the realm of laser micro drilling across various materials, benefiting future manufacturing endeavors.

Scanning laser ophthalmoscopy ‐ Basic optical principles

Scanning Laser Ophthalmoscopy (SLO) produces an ocular fundus image by moving a focused laser beam via scanning mirrors over the retina in a grid pattern and registering the reflected light from each scanned point. In confocal SLO, a pinhole is placed in front of the detector to cut off scattered or defocused light coming from outside the point of interest, which otherwise can blur the image. This results in a focused, high‐contrast image of a single tissue layer located at the focal plane. Tomographic information can be extracted by moving the plane of the pinhole. The use of various wavelengths allows for different applications, such as fluorescein angiography, indocyanine green angiography, and autofluorescence imaging. This lecture will present the basic principles of SLO, as well as discuss notable applications and variants of the technology.

Plasmon-enhanced optoacoustic transducer with Ecoflex thin film for broadband ultrasound generation using overdriven pulsed laser diode.

Ultrasonic transducers facilitate noninvasive biomedical imaging and therapeutic applications. Optoacoustic generation using nanoplasmonic structures provides a technical solution for highly efficient broadband ultrasonic transducer. However, bulky and high-cost nanosecond lasers as conventional excitation sources hinder a compact configuration of transducer. Here, we report a plasmon-enhanced optoacoustic transducer (PEAT) for broadband ultrasound generation, featuring an overdriven pulsed laser diode (LD) and an Ecoflex thin film. The PEAT module consists of an LD, a collimating lens, a focusing lens, and an Ecoflex-coated 3D nanoplasmonic substrate (NPS). The LD is overdriven above its nominal current and precisely modulated to achieve nanosecond pulsed beam with high optical peak power. The focused laser beam is injected on the NPS with high-density electromagnetic hotspots, which allows for the efficient plasmonic photothermal effect. The thermal expansion of Ecoflex finally generates broadband ultrasound. The overdriven pulsed LD achieves a maximum optical peak power of 40W, exceeding the average optical power of 3W. The thick Ecoflex-coated NPS exhibits an eightfold optoacoustic enhancement with a fractional bandwidth higher than 160% and a peak frequency of 2.5MHz. In addition, the optoacoustic amplitude is precisely controlled by the optical peak power or the laser pulse width. The PEAT-integrated microfluidic chip clearly demonstrates acoustic atomization by generating aerosol droplets at the air-liquid interface. Plasmon-enhanced optoacoustic generation using PEAT can provide an approach for compact and on-demand biomedical applications, such as ultrasound imaging and lab-on-a-chip technologies.

Photocatalytic activity of colloidal Bi–Si-based nanoparticles prepared by laser synthesis in liquid

A combination of laser ablation and laser irradiation by focused laser beam in liquid is used to prepare the Bi- and Si-based nanocolloids in water in a Bi:Si molar ratio of 12:1. The composition, structure, morphology, and optical properties of the obtained nanostructures are studied. The synthesized composite nanostructures are shown to consist mainly of bismuth oxycarbonate Bi2(CO3)O2 and bismuth silicate Bi12SiO20. The materials are tested in the decomposition of the model dye rhodamine B, including the stability of the catalyst and the opportunity of its regeneration by laser irradiation as well as in phenol decomposition when excited by LED with a wavelength of 375 nm. The opportunity to use the Bi–Si-based colloidal nanostructures for the selective photooxidation of 5-(hydroxymethyl)furfural is considered.